Goulart was reportedly engaged to businessman Marcelo Costa on August 2006. Although she mentioned being single during a February 2008 interview on Late Night with Conan O'Brien, she stated she was still with Costa in an interview for GQ Italia, November 2009.
Goulart, whose brother has type 1 diabetes, does charitable work, helping hospitals in her native Brazil to raise money to provide free insulin for diabetic children in need. She also has taken an active role with the Diabetes Research Institute (DRI) at the University of Miami, a recognized leader in cure-focused research. In 2009, Goulart became the DRI's international ambassador and in that role helps to promote the work of the DRI throughout her travels.
During an appearance on Late Night with Conan O'Brien in May 2006, O'Brien asked, "What kind of guy do you look for?", and Goulart simply replied "You."
On February 28, 2007, on a follow-up appearance on the show, O'Brien asked to dance with her, and Goulart then suggested dinner after the show. She mentioned that, "In Brazil we have a saying - You're married, but you're not dead."
Goulart appeared again on Late Night, this time on February 7, 2008. She brought O'Brien a Valentine's Day gift, which was later given away to an audience member, who ran with him to the backstage, for taking a good picture of O'Brien and Brian Williams. In the episode, she mentioned that she learned English by watching Woody Woodpecker cartoons.
Goulart appeared in an episode of Two And A Half Men.
She made a guest appearance in the thirteenth episode of season 3 of Entourage alongside fellow Angel Alessandra Ambrosio.
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